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Last episode of Space Runaway Ideon is a classic violent episode where they killed off every character. You can find that on YouTube.
Elfen Lied combines the kawaii (cute) and the gore and actually has a good story. The first 15 minutes is amazing stuff. Ninja Scroll, the original movie is pretty sick, perverted with great action.
Others to take a look at: Berserk, Hellsing, Ninja Resurrection, Evangelion (Death and Rebirth).
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