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You have to define "Downtown Atlanta"....if you just mean in Atlanta, then yes, the Four Seasons, imho, would be the most luxurious....however, it is in Midtown. In Buckhead it would be a toss up between the Ritz Carlton - Buckhead and the JW Marriott. If you are truly looking for downtown, then it would be the Ritz Carlton - Downtown Atlanta.
Hope this helps!
--T
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